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The theory of second-harmonic generation (SHG) that is due to quadrupole and magnetic-dipole second-order optical susceptibilities is developed for monochromatic, focused beams of arbitrary transverse mode structure and polarization character. The strength of SHG depends sensitively on the polarization character of the beam. © 1981 Optical Society of America.
D.S. Bethune, J.R. Lankard, et al.
The Journal of Chemical Physics
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